Fabrication of oxide pellets containing lumped Gd2O3 using Y2O3-stabilized ZrO2 for burnable absorber fuel applications

Qusai M. Mistarihi, Wooseong Park, Kyungseok Nam, Mohd Syukri Yahya, Yonghee Kim, Ho Jin Ryu

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Abstract

In this paper, the fabrication of novel burnable absorber fuel concepts with oxide pellets, containing either a lumped Gd2O3 rod, a mini-pellet, or a spherical particle in the centerline of the oxide pellet, is investigated to propose the lumped Gd2O3 burnable absorber fuel concept to improve nuclear fuel performance with longer fuel cycle lengths and better fuel utilization. The unique characteristic of the lumped Gd2O3 burnable absorber fuel is its high spatial self-shielding factor that reduces its burnout rate and, therefore, improves the reactivity control. Oxide pellets containing lumped Gd2O3 were fabricated by using a combination of cold isostatic pressing and microwave sintering at 1500°C to understand the potential technical issues in the fabrication of duplex burnable absorber fuel. The effect of the sintering temperature on the densification and phase transformation of 8 wt.% yttria-stabilized zirconia, a surrogate for UO2, was investigated. Spherical Gd2O3 particles were fabricated by the drip casting of a Gd2O3-based Na alginate solution. The fabrication of duplex oxide pellets by using presintered Gd2O3 mini-pellets resulted in internal cracks at the interface between the Gd2O3 and 8 wt.% yttria-stabilized zirconia layers because of the mismatch of their densification. However, the formation of interfacial cracks was eliminated by controlling the initial sintered density of the lumped Gd2O3.

Original languageEnglish
Pages (from-to)2141-2151
Number of pages11
JournalInternational Journal of Energy Research
Volume42
Issue number6
DOIs
Publication statusPublished - May 2018

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All Science Journal Classification (ASJC) codes

  • Renewable Energy, Sustainability and the Environment
  • Nuclear Energy and Engineering
  • Fuel Technology
  • Energy Engineering and Power Technology

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